Charles S. Cockell

Astrobiology


Скачать книгу

The exception to this is glycine. The best, and most iconic, way to explain this is with your hands. Place your left hand on a table palm down. Now place your right hand on top of it, palm down. They don't exactly overlap. Your left hand's thumb sticks out to the right, your right hand's thumb to the left. That is because they are mirror images. They are non-superimposable (Figure 4.6).

Image described by caption.

       Figure 4.6 Chirality illustrated with hands and the generic structure for amino acids.

      Source: Reproduced with permission of wikicommons, https://commons.wikimedia.org/wiki/File:Chirality_with_hands.svg.

Image described by caption and surrounding text.

       Figure 4.7 Chiral molecules rotate polarized light in particular directions. Schematically, the rotation of light to the left (levorotation) is shown here with the amino acid, L-alanine.

      Discussion Point: Life with a Different Chirality

      Why are almost all amino acids used in life found in the L form? Is it possible to construct life forms in which D-amino acids are the dominant amino acids in protein-like structures? Or would life elsewhere also be biased toward L-amino acids? We return to this when we discuss astrochemistry (Chapter 10) and after that chapter you might like to revisit this question. Life on Earth uses D-sugars, but what about a life form that uses L-sugars? What information can you gather to shed light on why life on Earth chose L-amino acids? What range of problems and even advantages could you think of for a lifeform that used a racemic mix of D- and L-amino acids in its biochemical architecture? In Figure 4.8, you can see the four possible ways one might construct a life form. Is there a reason why Gertie is made the way she is or were the three other forms possible?

      Bonner, W.A. (1991). The origin and amplification of biomolecular chirality. Origins of Life and Evolution of Biospheres 21: 59–111.

      Breslow, R. and Cheng, Z.-L. (2009). On the origin of terrestrial homochirality for nucleosides and amino acids. Proceedings of the National Academy of Sciences of the United States of America 106: 9144–9146.

Gertie the L-sugar aardvark (left) and Gertie the D-amino acid, L-sugar aardvark (right).

       Figure 4.8 Different chiralities of life? Gertie the aardvark is a rescued aardvark. She is made of L-amino acids and D-sugars. Is it theoretically possible for Gertie to exist in the three other chiral combinations of L- and D-amino acids or L- and D-sugars?

      Now an interesting thing about life on Earth is that almost all the amino acids used in life are of the L form. The D form is very rare, although D-amino acids are found in the cell membranes of bacteria. They reappear in the next chapter. The reason why life predominantly uses one form of amino acids is not fully understood, but it might have something to do with molecular recognition. As many biochemical interactions involve one molecule slotting into another to carry out chemical reactions, a system of life that was a mix of L and D forms would cause great complexity because we would need proteins with active sites that could recognize either the L or D form of molecules. It seems plausible to speculate that once a biochemical architecture emerged that had a preponderance to use either the L or D form, then that choice would have been perpetuated and amplified. Life on Earth developed a biochemistry based on the L form. Later in the textbook, we explore the possibility that the preference for the L form in life was caused by a pre-existing enantiomeric excess of L forms of amino acids in the prebiotic compounds from which life originated.

Image described by caption.

       Figure 4.9 The molecular structure of the sugars: glucose, fructose, and ribose. The figure shows the numbering convention on the carbon atoms. Note that the carbon atoms within the rings are not indicated with the letter “C,” but occur where the numbers are shown.

      A sugar with six carbon atoms is called a hexose (hence despite their different structures, glucose and fructose are hexose sugars, as they both contain six carbon atoms). A sugar with five carbon atoms is called a pentose. Ribose is such an example (Figure 4.9). This sugar is found in the structure of ribonucleic acid (RNA) as part of the repeating ribose–phosphate backbone.

      Sugars join through a glycosidic bond to form chains, analogous to the peptide bonds in proteins. O-glycosidic bonds are oxygen-bridged links between sugar molecules (Figure 4.10). Figure 4.10 shows the example of maltose formed by a link between the –OH bond of one glucose (the 4 carbon position) and the hemiacetal group of another glucose (that is the carbon with an –OH group and a link to the oxygen atom in the sugar ring – the 1 carbon position in glucose). This explains why they are sometimes called 1,4 glycosidic linkages. Alternatively, a link between the 1 carbon of a glucose molecule and the 2 carbon of a fructose molecule (the hemiacetal carbon) produces the sugar sucrose (a 1,2 glycosidic link). Like the formation of the peptide bond in proteins, glycosidic linkages are condensation reactions in which a water molecule is lost during the reaction.

Image described by caption.

       Figure 4.10 Glycosidic bonds allow sugar molecules to be linked together. In this case, two glucose molecules have linked together to form the two-sugar molecule maltose. By adding further units, we can produce polysaccharides (carbohydrates).

      A further subtlety, but one crucial for life, is the way in which the glycosidic links are formed. For example, the 1,4 glycosidic link can exist in a 1,4 alpha or 1,4 beta form. The 1,4 alpha form occurs when the –OH group is below the plane of the glucose ring (alpha glucose), while the beta form occurs when the –OH is above the ring (beta glucose) (Figure 4.11). The differences between these two forms of glucose may seem a trivial point of fact, but the consequences of the links formed between them are immense. In the former case, the linking together of many alpha glucose molecules