William M. White

Geochemistry


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the amount of work done does not depend only on the initial and final values of T and P; it depends on the path taken. Heat is also not a state function, not an exact differential, and is also path dependent. Path dependent functions always have inexact differentials; path independent functions always have exact differentials.

      On a less mathematical level, let's consider how the work and heat will vary in a transformation of a system, say from state 1 to state 2. Imagine that we burn gasoline in an open container. In this case, in the transformation from state 1 (gasoline) to state 2 (combustion products of gasoline), energy is given up by the system only as heat. Alternatively, we could burn the gasoline in an engine and recover some of the energy as work (expansion of the volume of the cylinder resulting in motion of the piston). The end states of these two transformations are the same, but the amount of heat released and work done varies, depending on the path we took. Thus, neither work nor heat can be state functions. Energy is a state function, is path independent, and is an exact differential. Whether we burn the gasoline in an open container or an engine, the energy released will be the same. Herein lies the significance for thermodynamics of Joule's discovery: that the sum of heat and work is independent of the path taken even though, independently, work and heat are not.

      2.6.1 Statement

      The second law may be stated in a number of ways:

Schematic illustration of a gas-filled box with a removable partition. When the partition is removed, the gases mix. Entropy increases during this process.

      Heat cannot be entirely extracted from a body and turned into work (thus car engines always have cooling systems).

      Every system left to itself will, on average, change toward a condition of maximum probability.

      Introducing a new state function S called entropy, we may state the second law as:

      The entropy of the universe always increases.

      In colloquial terms we could say:

      You can't shovel manure into the rear end of a horse and expect to get hay out its mouth.

      The second law codifies some of our everyday experience. The first law would not prevent us from using a horse to manufacture hay from manure. It only says we cannot get more joules worth of hay out than we put in as manure. We would search in vain for any other physical law that prohibited this event. Yet our experience shows that it will not happen. Indeed, this event is so improbable that we find it comical. Similarly, we know that we can convert gasoline and oxygen to carbon dioxide and water in an internal combustion engine and use the resulting energy to drive a vehicle down the road. But adding CO2 and water to the engine and pushing the car backwards down the street does not produce gasoline and oxygen, although such a result violates no other law of physics. The second law states that there is a natural direction in which reactions will tend to proceed. This direction is inevitably that of higher entropy of the system and its surroundings.

      2.6.2 Statistical mechanics: a microscopic perspective of entropy

      Whereas energy is a property for which we gain an intuitive feel through everyday experience, the concept of entropy is usually more difficult to grasp. Perhaps the best intuitive understanding of entropy can be obtained from the microscopic viewpoint of statistical mechanics. So for that reason, we will make the first of several brief excursions into the world of atoms, molecules, and quanta.

      Let's return to our box of gas and consider what happens on a microscopic scale when we remove the partition. To make things tractable, we'll consider that each gas consists of only two molecules, so there are four all together, two red and two black. For this thought experiment, we will keep track of the individual molecules so we label them 1red, 2red, 1black, 2black. Before we removed the partition, the red molecules were on one side and the black ones on the other. Our molecules have some thermal energy, so they are free to move around. So by removing the partition, we are essentially saying that each molecule is equally likely to be found in either side of the box.

Schematic illustration of the possible distribution of molecules of a red and a black gas in a box before (a) and (b) after removal of a partition separating them.

      Now let's look at this process on a microscopic scale. We have already mentioned that temperature is related to internal energy. As we shall see, this relationship will differ depending on the nature and mass of the material of interest, but since our blocks are of identical size and composition, we can assume that temperature and energy are directly related in this case. Suppose that before we remove the insulation, the left block has one unit of energy and the right one has five units (we can think of these as quanta, but this is not necessary). The question